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[1]张 君,王新锋*,张英南,等.北京市区冬季颗粒态有机硝酸酯的污染特征与生成[J].地球化学,2020,49(03):252-261.[doi:10.19700/j.0379-1726.2020.01.010]
 ZHANG Jun,WANG Xin-feng*,ZHANG Ying-nan,et al.Pollution characteristics and formation of particulate organic nitrates in winter in Beijing City[J].Geochimica,2020,49(03):252-261.[doi:10.19700/j.0379-1726.2020.01.010]



[1] Fry J L, Draper D C, Zarzana K J, Campuzano-Jost P, Day D A, Jimenez J L, Brown S S, Cohen R C, Kaser L, Hansel A, Cappellin L, Karl T, Hodzic Roux A, Turnipseed A, Cantrell C, Lefer B L, Grossberg N. Observations of gas- and aerosol-phase organic nitrates at BEACHON-RoMBAS 2011[J]. Atmos Chem Phys, 2013, 13(17): 8585-8605.
[2] Rollins A W, Browne E C, Min K E, Pusede S E, Wooldridge P J, Gentner D R, Goldstein A H, Liu S, Day D A, Russell L M, Cohen R C. Evidence for NOx control over nighttime SOA formation[J]. Science, 2012, 337(6099): 1210-1212.
[3] Xu L, Suresh S, Guo H, Weber R J, Ng N L. Aerosol characterization over the southeastern United States using high-resolution aerosol mass spectrometry: Spatial and seasonal variation of aerosol composition and sources with a focus on organic nitrates[J]. Atmos Chem Phys, 2015, 15(13): 7307-7336.
[4] Horowitz L W, Fiore A M, Milly G P, Cohen R C, Perring A, Wooldridge P J, Hess P G, Emmons L K, Lamarque J-F. Observational constraints on the chemistry of isoprene nitrates over the eastern United States[J]. J Geophys Res, 2007, 112(D12S08): 1-13.
[5] Xiong F, Mcavey K M, Pratt K A, Groff C J, Hostetler M A, Lipton M A, Starn T K, Seeley J V, Bertman S B, Teng A P, Crounse J D, Nguyen T B, Wennberg P O, Misztal P K, Goldstein A H, Guenther A B, Koss A R, Olson K F, De Gouw J A, Baumann K, Edgerton E S, Feiner P A, Zhang L, Miller D O, Brune W H, Shepson P B. Observation of isoprene hydroxynitrates in the southeastern United States and implications for the fate of NOx[J]. Atmos Chem Phys, 2015, 15(19): 11257-11272.
[6] Renbaum L H, Smith G D. Organic nitrate formation in the radical-initiated oxidation of model aerosol particles in the presence of NOx[J]. Phys Chem Chem Phys, 2009, 11(36): 8040-8047.
[7] Perring A E, Pusede S E, Cohen R C. An observational perspective on the atmospheric impacts of alkyl and multifunctional nitrates on ozone and secondary organic aerosol[J]. Chem Rev, 2013, 113(8): 5848-5870.
[8] 顾芳婷, 胡敏, 郑竞, 郭松. 大气颗粒物中有机硝酸酯的研究进展[J]. 化学进展, 2017, 29(9): 962-969.
Gu Fang-ting, Hu Min, Zheng Jing, Guo Song. Research progress on particulate organonitrates[J]. Prog Chem, 2017, 29(9): 962-969 (in Chinese with English abstract).
[9] Lee B H, Mohr C, Lopez-Hilfiker F D, Lutz A, Hallquist M, Lee L, Romer P, Cohen R C, Iyer S, Kurten T, Hu W W, Day D A, Campuzano-Jost P, Jimenez J L, Xu L, Ng N L, Guo H Y, Weber R J, Wild R J, Brown S S, Koss A, De Gouw J, Olson K, Goldstein A H, Seco R, Kim S, Mcavey K, Shepson P B, Starn T, Baumann K, Edgerton E S, Liu J M, Shilling J E, Miller D O, Brune W, Schobesberger S, D’ambro E L, Thornton J A. Highly functionalized organic nitrates in the southeast United States: Contribution to secondary organic aerosol and reactive nitrogen budgets[J]. Proc Natl Acad Sci USA, 2016, 113(6): 1516-1521.
[10] Kiendler-Scharr A, Mensah A A, Friese E, Topping D, Nemitz E, Prevot A S H, Aijala M, Allan J, Canonaco F, Canagaratna M, Carbone S, Crippa M, Dall Osto M, Day D A, De Carlo P, Di Marco C F, Elbern H, Eriksson A, Freney E, Hao L, Herrmann H, Hildebrandt L, Hillamo R, Jimenez J L, Laaksonen A, Mcfiggans G, Mohr C, O’dowd C, Otjes R, Ovadnevaite J, Pandis S N, Poulain L, Schlag P, Sellegri K, Swietlicki E, Tiitta P, Vermeulen A, Wahner A, Worsnop D, Wu H C. Ubiquity of organic nitrates from nighttime chemistry in the European submicron aerosol[J]. Geophys Res Lett, 2016, 43(14): 7735-7744.
[11] Chen X R, Wang H C, Lu K D. Simulation of organic nitrates in Pearl River Delta in 2006 and the chemical impact on ozone production[J]. Sci China Earth Sci, 2018, 61(2): 228-238.
[12] Pye H O T, Luecken D J, Xu L, Boyd C M, Ng N L, Baker K R, Ayres B R, Bash J O, Baumann K, Carter W P L, Edgerton E, Fry J L, Hutzell W T, Schwede D B, Shepson P B. Modeling the current and future roles of particulate organic nitrates in the southeastern United States[J]. Environ Sci Technol, 2015, 49(24): 14195-14203.
[13] Wang Y J, Hu M, Guo S, Wang Y C, Zheng J, Yang Y D, Zhu W F, Tang R Z, Li X, Liu Y, Le Breton M, Du Z F, Shang D J, Wu Y S, Wu Z J, Song Y, Lou S R, Hallquist M, Yu J Z. The secondary formation of organosulfates under interactions between biogenic emissions and anthropogenic pollutants in summer in Beijing[J]. Atmos Chem Phys, 2018, 18(14): 10693-10713.
[14] Li R, Wang X F, Gu R R, Lu C Y, Zhu F P, Xue L K, Xie H J, Du L, Chen J M, Wang W X. Identification and semi-quantification of biogenic organic nitrates in ambient particulate matters by UHPLC/ESI-MS[J]. Atmos Environ, 2018, 176: 140-147.
[15] He Q F, Ding X, Wang X M, Yu J Z, Fu X X, Liu T Y, Zhang Z, Xue J, Chen D H, Zhong L J, Donahue N M. Organosulfates from pinene and isoprene over the Pearl River Delta, South China: seasonal variation and implication in formation mechanisms[J]. Environ Sci Technol, 2014, 48(16): 9236- 9245.
[16] 马乾坤, 成春雷, 李梅, 黄祖照, 桂华侨, 张礁石, 周振. 北京郊区秋季灰霾天气下细颗粒物化学成分及其混合特征研究[J]. 地球化学, 2019, 48(2): 195-203.
Ma Qian-kun, Cheng Chun-lei, Li Mei, Huang Zu-zhao, Gui Hua-qiao, Zhang Jiao-shi, Zhou Zhen. Chemical composition and mixing state of single particles during the haze period at a Beijing suburb site[J]. Geochimica, 2019, 48(2): 195-203 (in Chinese with English abstract).
[17] Wang X F, Chen J M, Sun J F, Li W J, Yang L X, Wen L, Wang W X, Wang X M, Collett Jr J L, Shi Y, Zhang Q Z, Hu J T, Yao L, Zhu Y H, Sui X, Sun X M, Mellouki A. Severe haze episodes and seriously polluted fog water in Ji’nan, China[J]. Sci Total Environ, 2014, 493: 133-137.
[18] 汪午, 王省良, 李黎, 张东平, 王扬君, 盛国英, 傅家谟. 天然源二次有机气溶胶的研究进展[J]. 地球化学, 2008, 37(1): 77-86.
Wang Wu, Wang Sheng-liang, Li Li, Zhang Dong-ping, Wang Yang-jun, Sheng Guo-ying, Fu Jia-mo. Advances in biogenic secondary organic aerosols[J]. Geochimica, 2008, 37(1): 77-86 (in Chinese with English abstract).
[19] Wang T, Nie W, Gao J, Xue L K, Gao X M, Wang X F, Qiu J, Poon C N, Meinardi S, Blake D, Wang S L, Ding A J, Chai F H, Zhang Q Z, Wang W X. Air quality during the 2008 Beijing Olympics: secondary pollutants and regional impact[J]. Atmos Chem Phys, 2010, 10(16): 7603-7615.
[20] 郑玫, 闫才青, 李小滢, 王雪松, 张远航. 二次有机气溶胶估算方法研究进展[J]. 中国环境科学, 2014, 34(3): 555-564.
Zheng Mei, Yan Cai-qing, Li Xiao-ying, Wang Xue-song, Zhang Yuan-hang. A review of methods for quantifying secondary organic aerosol[J]. China Environ Sci, 2014, 34(3): 555-564 (in Chinese with English abstract).
[21] Hu W W, Hu M, Hu W, Jimenez J L, Yuan B, Chen W T, Wang M, Wu Y S, Chen C, Wang Z B, Peng J F, Zeng L M, Shao M. Chemical composition, sources, and aging process of submicron aerosols in Beijing: Contrast between summer and winter[J]. J Geophys Res Atmos, 2016, 121(4): 1955-1977.
[22] Chang W L, Bhave P V, Brown S S, Riemer N, Stutz J, Dabdub D. Heterogeneous atmospheric chemistry, ambient measurements, and model calculations of N2O5: A review[J]. Aerosol Sci Technol, 2011, 45(6): 665-695.
[23] Sander S P, Golden D M, Kurylo M J, Moortgat G K, Wine P H, Ravishankara A R, Kolb C E, Molina M J, Finlayson-Pitts B J, Huie R E, Orkin V L. Chemical kinetics and photochemical data for use in atmospheric studies evaluation number 15[J]. Jet Propuls Lab, 2006, 45: 665-695.
[24] Fry J L, Kiendler-Scharr A, Rollins A W, Brauers T, Brown S S, Dorn H P, Dubé W P, Fuchs H, Mensah A, Rohrer F, Tillmann R, Wahner A, Wooldridge P J, Cohen R C. SOA from limonene: Role of NO3 in its generation and degradation[J]. Atmos Chem Phys, 2011, 11(8): 3879-3894.
[25] Jenkin M E, Saunders S M, Pilling M J. The tropospheric degradation of volatile organic compounds: A protocol for mechanism development[J]. Atmos Environ, 1997, 31(1): 81-104.
[26] Saunders S M, Jenkin M E, Derwent R G, Pilling M J. Protocol for the development of the Master Chemical Mechanism, MCM v3 (Part A): Tropospheric degradation of non-aromatic volatile organic compounds[J]. Atmos Chem Phys, 2003, 3(1): 161-180.
[27] Xue L K, Wang T, Gao J, Ding A J, Zhou X H, Blake D R, Wang X F, Saunders S M, Fan S J, Zuo H C, Zhang Q Z, Wang W X. Ground-level ozone in four Chinese cities: Precursors, regional transport and heterogeneous processes[J]. Atmos Chem Phys, 2014, 14(23): 13175-13188.
[28] Zhang L, Brook J R, Vet R. A revised parameterization for gaseous dry deposition in air-quality models[J]. Atmos Chem Phys, 2003, 3(6): 2067-2082.
[29] Chen X R, Wang H C, Lu K D. Simulation of organic nitrates in Pearl River Delta in 2006 and the chemical impact on ozone production[J]. Sci China Earth Sci, 2018, 61(2): 228-238.
[30] Perring A E, Bertram T H, Wooldridge P J, Fried A, Heikes B G, Dibb J, Crounse J D, Wennberg P O, Blake N J, Blake D R, Brune W H, Singh H B, Cohen R C. Airborne observations of total RONO2: New constraints on the yield and lifetime of isoprene nitrates[J]. Atmos Chem Phys, 2009, 9(4): 1451- 1463.
[31] Reyes-Villegas E, Priestley M, Ting Y C, Haslett S, Bannan T, Le Breton M, Williams P I, Bacak A, Flynn M J, Coe H, Percival C, Allan J D. Simultaneous aerosol mass spectrometry and chemical ionisation mass spectrometry measurements during a biomass burning event in the UK: Insights into nitrate chemistry[J]. Atmos Chem Phys, 2018, 18(6): 4093-4111.
[32] Rinne H J I, Guenther A B, Greenberg J P, Harley P C. Isoprene and monoterpene fluxes measured above Amazonian rainforest and their dependence on light and temperature[J]. Atmos Environ, 2002, 36(14): 2421-2426.
[33] Cheng Y, Li S M. Nonderivatization analytical method of fatty acids and cis-pinonic acid and its application in ambient PM2.5 aerosols in the greater Vancouver Area in Canada[J]. Environ Sci Technol, 2005, 39(7): 2239-2246.
[34] Schauer J J, Kleeman M J, Cass G R, Simoneit B R T. Measurement of emissions from air pollution sources. 4. C1-C27 organic compounds from cooking with seed oils[J]. Environ Sci Technol, 2002, 36(4): 567-575.
[35] Rogge W F, Hildemann L M, Mazurek M A, Cass G R, Simonelt B R T. Sources of fine organic aerosol. 1. charbroilers and meat cooking operations[J]. Environ Sci Technol, 1991, 25(6): 1112-1125.
[36] Docherty K S, Ziemann P J. Reaction of oleic acid particles with NO3 radicals: Products, mechanism, and implications for radical-initiated organic aerosol oxidation[J]. J Phys Chem A, 2006, 110(10): 3567-3577.
[37] Berkemeier T, Ammann M, Mentel T F, Poschl U, Shiraiwa M. Organic nitrate contribution to new particle formation and growth in secondary organic aerosols from alpha-Pinene ozonolysis[J]. Environ Sci Technol, 2016, 50(12): 6334-6342.
[38] Zhang Y N, Sun J J, Zheng P G, Chen T S, Liu Y H, Han G X, Simpson I J, Wang X F, Blake D R, Li Z Y, Yang X, Qi Y B, Wang Q, Wang W X, Xue L K. Observations of C1-C5 alkyl nitrates in the Yellow River Delta, northern China: Effects of biomass burning and oil field emissions[J]. Sci Total Environ, 2019, 656: 129-139.
[39] Sun J J, Li Z Y, Xue L K, Wang T, Wang X F, Gao J, Nie W, Simpson I J, Gao R, Blake D R, Chai F H, Wang W X. Summertime C1-C5 alkyl nitrates over Beijing, northern China: Spatial distribution, regional transport, and formation mechanisms[J]. Atmos Res, 2018, 204: 102-109.


收稿日期(Received): 2019-08-24; 改回日期(Revised): 2019-12-04; 接受日期(Accepted): 2019-12-11
基金项目: 国家自然科学基金(91544213, 41775118); 北京市科委首都蓝天行动培育专项(Z181100005418015)
作者简介: 张君(1994-), 女, 硕士研究生, 环境科学与工程专业。E-mail: zhangjun1994321@163.com
* 通讯作者(Corresponding author): WANG Xin-feng, E-mail: xinfengwang@sdu.edu.cn; Tel: +86-532-58631963

更新日期/Last Update: 2020-06-20